بهینه سازی آب آلوده به پارا نیترو فنل توسط فناوری پلاسمای غیر حرارتی و ازن زنی به روش سطح پاسخ

نوع مقاله : پژوهشی اصیل (کامل)

نویسندگان
امیرحسین خورشیدی 1
فرهاد قادری 2
1 دانشجوی کارشناسی ارشد دانشگاه صنعتی نوشیروانی بابل
2 دانشگاه صنعتی نوشیروانی بابل
10.22034/23.5.13
چکیده
آلاینده‌های آلی و غیرقابل تجزیه زیادی وجود دارند که در نتیجه توسعه صنعتی تولید شده اند، از جمله ترکیبات نفتی. استفاده از فناوری پلاسما برای تصفیه فاضلاب به دلیل پتانسیل آن برای حذف موثر طیف گسترده ای از آلاینده ها مورد توجه روزافزون قرار گرفته است. از طرفی ازن‌ به عنوان یک فرآیند اکسیدکننده قوی، مزایای زیادی در تصفیه فاضلاب دارد و پتانسیل استفاده عملی در مقیاس صنعتی را دارد. استفاده از فرآیند ازن‌زنی در کنار تکنولوژی پلاسما علاوه بر کاربردی که در بالابردن سرعت و کم کردن زمان تصفیه آلاینده‌های آلی همچون پارانیتروفنول دارد، در بالا بردن راندمان حذف، کاهش مصرف انرژی که منجر به اقتصادی‌تر شدن این فرآیند است نیز کمک می‌کند. در تحقیق کنونی، پس از بررسی راندمان حذف پارانیتروفنول با استفاده از فرآیند پلاسما-ازن در شرایط مختلف، تاثیر متغیرهای موثر در این تکنیک نیز مورد بررسی قرار گرفت. سپس مکانیزم احتمالی حذف پارانیتروفنول با استفاده از پلاسما و ازن نیز مورد تجزیه و تحلیل قرار گرفت. همچنین با توجه به اثرات هم افزایی و کاهنده و اثرات همزمان متغیرها، شرایط بهینه حذف آلاینده‌ها با استفاده از مدل درجه دوم مبتنی بر تحلیل واریانس (ANOVA) و تعیین سطح معنی داری هر متغیر بالاترین راندمان حذف (بیش از 95٪) در ولتاژ اعمالی 14 kV، شدت جریان اکسیژن 6 l/h، pH اولیه 10، مدت زمان فرآیند 6 دقیقه، غلظت اولیه PNP mg/l 200 به دست آمد.

کلیدواژه‌ها

موضوعات

عنوان مقاله English

Optimization of P-nitrophenol-Contaminated Water by Non-thermal Plasma Technology and Ozonation by Response Surface Method

نویسندگان English

A.h Khourshidi 1
F. Qaderi 2
1 Master's student of Noshirvani University of Technology, Babol
2 Babol Noshirvani University of Technology
چکیده English

Industrial progress has ushered in the production of a diverse array of pollutants, encompassing both organic and non-biodegradable substances, such as hydrocarbon compounds derived from petroleum. As the discernible environmental ramifications of these pollutants continue to escalate, the quest for efficacious methodologies for wastewater remediation assumes paramount importance. Among the emergent technologies, plasma technology has garnered considerable acclaim due to its capacity to obliterate a myriad of pollutants. Plasma, which ensues from the application of high voltage to either a gaseous or liquid medium, engenders profoundly reactive species capable of dismantling intricate organic compounds. Similarly, ozone, an exceedingly potent oxidizing agent, has long commanded recognition for its aptitude in the degradation of pollutants. Its robust oxidative attributes render it an invaluable instrument in the realm of wastewater treatment. Ozone treatment entails the infusion of ozone gas into the contaminated aqueous medium, whereupon it engages pollutants in a transformative reaction, rendering them into less deleterious byproducts. By amalgamating the ozonation process with plasma technology, we can harness the merits of both modalities and achieve synergistic effects. This hybridized approach proffers several advantages vis-à-vis individual treatment methodologies, including augmented pollutant removal efficiency, diminished treatment duration, and amplified energy efficiency. The plasma-ozonation process exploits plasma's propensity for the generation of reactive species, capable of reacting with the organic constituents in wastewater. The ensuing ozonation phase augments the degradation of these constituents, engendering a more efficacious and comprehensive removal process. Prior investigations have scrutinized the efficacy of ozone and plasma in isolation for the eradication of p-nitrophenol, a ubiquitous organic pollutant encountered in industrial wastewater. These inquiries have methodically examined various parameters to ascertain their influence on pollutant removal efficiency. Factors such as applied voltage, ozone dosage, initial pH, reaction duration, and initial solution concentration have been subjected to meticulous scrutiny to optimize the treatment regimen. In the present study, we have devised an innovative mathematical model to probe the interplay between these two independent variables: plasma technology and ozonation. The model incorporates a quadratic equation and employs analysis of variance (ANOVA) to gauge the significance of each variable and discern the optimal conditions for pollutant removal. Through scrutiny of the model, we have ascertained that the pinnacle of removal efficiency, surpassing 95%, materializes under specific parameters. These parameters encompass an applied voltage of 14 kV, an oxygen flow rate of 6 L/min, an initial pH of 10, a reaction duration of 6 minutes, and an initial concentration of 200 mg/L. These revelations offer valuable insights into the operational parameters that yield superlative results for pollutant removal within the context of the plasma-ozonation process. The efficacious integration of ozone and plasma technologies in wastewater treatment proffers a promising panacea for the elimination of p-nitrophenol pollutants and sundry other organic constituents. By fine-tuning the process parameters in alignment with the model's recommendations, we can attain exceptional levels of pollutant elimination whilst concurrently minimizing energy consumption and treatment duration. This research significantly contributes to the perennial endeavors aimed at fashioning sustainable and efficient remedies for industrial wastewater treatment, endowing valuable perspectives for their future deployment and widescale application in industrial settings.





کلیدواژه‌ها English

Wastewater treatment
AOPs
non-thermal plasma
Ozonation
PNP
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2. Zhao B, Mele G, Pio I, Li J, Palmisano L, Vasapollo G. Degradation of 4-nitrophenol (4-NP) using Fe–TiO2 as a heterogeneous photo-Fenton catalyst. J Hazard Mater. 2010 Apr 15;176(1–3):569–74.
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6. Yan X, Yi C, Wang Y, Cao W, Mao D, Ou Q, et al. Multi-catalysis of nano-zinc oxide for bisphenol A degradation in a dielectric barrier discharge plasma system: Effect and mechanism. Sep Purif Technol. 2020 Jan 16;231:115897.
7. Sarkar P, Dey A. 4-Nitrophenol biodegradation by an isolated and characterized microbial consortium and statistical optimization of physicochemical parameters by Taguchi Methodology. J Environ Chem Eng. 2020 Oct 1;8(5):104347.
8. Zhao C, Xue L, Zhou Y, Zhang Y, Huang K. A microwave atmospheric plasma strategy for fast and efficient degradation of aqueous p-nitrophenol. J Hazard Mater. 2021 May 5;409:124473.
9. Farzinfar B, Qaderi F. Synergistic degradation of aqueous p-nitrophenol using DBD plasma combined with ZnO photocatalyst. Process Saf Environ Prot [Internet]. 2022 Dec;168(August):907–17. Available from: https://doi.org/10.1016/j.psep.2022.10.060
10. Azerrad SP, Isaacs M, Dosoretz CG. Integrated treatment of reverse osmosis brines coupling electrocoagulation with advanced oxidation processes. Chem Eng J [Internet]. 2019 Jan 15 [cited 2023 May 20];356:771–80. Available from: https://linkinghub.elsevier.com/retrieve/pii/S1385894718317856
11. Kaplan A, Mamane H, Lester Y, Avisar D. Trace Organic Compound Removal from Wastewater Reverse-Osmosis Concentrate by Advanced Oxidation Processes with UV/O3/H2O2. Materials (Basel) [Internet]. 2020 Jun 19 [cited 2023 May 20];13(12):2785. Available from: https://www.mdpi.com/1996-1944/13/12/2785/htm
12. Giannoulia S, Triantaphyllidou IE, Tekerlekopoulou AG, Aggelopoulos CA. Mechanisms of Individual and Simultaneous Adsorption of Antibiotics and Dyes onto Halloysite Nanoclay and Regeneration of Saturated Adsorbent via Cold Plasma Bubbling. Nanomaterials [Internet]. 2023 Jan 1 [cited 2023 May 20];13(2):341. Available from: https://www.mdpi.com/2079-4991/13/2/341/htm
13. Deng Y, Zhao R. Advanced Oxidation Processes (AOPs) in Wastewater Treatment. Curr Pollut Reports [Internet]. 2015 Sep 18 [cited 2023 May 20];1(3):167–76. Available from: https://link.springer.com/article/10.1007/s40726-015-0015-z
14. Iakovides IC, Michael-Kordatou I, Moreira NFF, Ribeiro AR, Fernandes T, Pereira MFR, et al. Continuous ozonation of urban wastewater: Removal of antibiotics, antibiotic-resistant Escherichia coli and antibiotic resistance genes and phytotoxicity. Water Res [Internet]. 2019 Aug;159:333–47. Available from: https://doi.org/10.1016/j.watres.2019.05.025
15. Hou X, Qiu Y, Yuan E, Li F, Li Z, Ji S, et al. Promotion on light olefins production through modulating the reaction pathways for n-pentane catalytic cracking over ZSM-5 based catalysts. Appl Catal A Gen. 2017 Aug 5;543:51–60.
16. Meijide J, Rosales E, Pazos M, Sanromán MA. p-Nitrophenol degradation by electro-Fenton process: Pathway, kinetic model and optimization using central composite design. Chemosphere. 2017 Oct 1;185:726–36.
17. Martins RC, Rossi AF, Quinta-Ferreira RM. Fenton’s oxidation process for phenolic wastewater remediation and biodegradability enhancement. J Hazard Mater. 2010 Aug 15;180(1–3):716–21.
18. Lin J, Hu H, Gao N, Ye J, Chen Y, Ou H. Fabrication of GO@MIL-101(Fe) for enhanced visible-light photocatalysis degradation of organophosphorus contaminant. J Water Process Eng [Internet]. 2020 Feb;33(October 2019):101010. Available from: https://doi.org/10.1016/j.jwpe.2019.101010
19. Yang T, Peng J, Zheng Y, He X, Hou Y, Wu L, et al. Enhanced photocatalytic ozonation degradation of organic pollutants by ZnO modified TiO2 nanocomposites. Appl Catal B Environ [Internet]. 2018 Feb 1 [cited 2023 Apr 24];221:223–34. Available from: https://linkinghub.elsevier.com/retrieve/pii/S0926337317308640
20. Shang K, Li W, Wang X, Lu N, Jiang N, Li J, et al. Degradation of p-nitrophenol by DBD plasma/Fe2+/persulfate oxidation process. Sep Purif Technol. 2019 Jul 1;218:106–12.
21. Hama Aziz KH, Mahyar A, Miessner H, Mueller S, Kalass D, Moeller D, et al. Application of a planar falling film reactor for decomposition and mineralization of methylene blue in the aqueous media via ozonation, Fenton, photocatalysis and non-thermal plasma: A comparative study. Process Saf Environ Prot. 2018 Jan 1;113:319–29.
22. Yu Q, Gao Y, Tang X, Yi H, Zhang R, Zhao S, et al. Removal of NO from flue gas over HZSM-5 by a cycling adsorption-plasma process. Catal Commun [Internet]. 2018;110(December 2017):18–22. Available from: https://doi.org/10.1016/j.catcom.2018.02.025
23. Liu Y, Wang C, Huang K, Miruka AC, Dong A, Guo Y, et al. Degradation of glucocorticoids in water by dielectric barrier discharge and dielectric barrier discharge combined with calcium peroxide: performance comparison and synergistic effects. J Chem Technol Biotechnol. 2019;94(11):3606–17.
24. Xin YY, Zhou L, Ma K ke, Lee J, Qazi HIA, Li HP, et al. Removal of bromoamine acid in dye wastewater by gas-liquid plasma: The role of ozone and hydroxyl radical. J Water Process Eng. 2020 Oct 1;37:101457.
25. Shang K, Wang X, Li J, Wang H, Lu N, Jiang N, et al. Synergetic degradation of Acid Orange 7 (AO7) dye by DBD plasma and persulfate. Chem Eng J [Internet]. 2017 Mar [cited 2022 Jun 11];311:378–84. Available from: https://linkinghub.elsevier.com/retrieve/pii/S1385894716316655
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مهندسی عمران مدرس
دوره 23، شماره 5
مهر و آبان 1402
صفحه 179-193